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I have a modded PSP 2000 and after downloading the PSX game you have to convert the ISO to EBOOT.PBP using POPSConv.exe ad after conversion you place the eboot into the PSP/GAME folder. If you have PSX game disc check out http://www.psxpsp.com/ps1-support-help.php. Depending on your converter you may have to make config changes and or use with an emulator.
first you need custom firmware to play iso files, second the psx2psp is to change playstation 1 games into psp eboots not psp games, the iso is all you need for psp games if you have custom firmware, you just need to create a folder called ISO in the root of your memory stick and put the iso files in there