I think you may just have a dead battery. The batteries on the iPod last a long time but they do go bad after years of use.
Occasionally a battery will die almost immediately without warning.
Also, use an AC wall charger to verify it's actually being charged.
USB cables work for transferring music, but are a weak source for charging. If you need a battery click here or check ebay they are fairly inexpensive to replace.
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What model Ipod do you have? Have you tried resetting your Ipod to its factory default settings with the Ipod reset tool?
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