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The first way is uncheck the songs you want to delete on iTunes and then sync iTunes with ipod again, then the songs you want to delete will lose from iPod.
The second way is use leawo iTransfer to delete songs from iPod, the way is connect iPod to leawo iTransfer, then right click on the music you want to delete from iPod on leawo iTransfer to choose "Delete", then the music will be deleted soon. However, this tool can only work on Windows computer.
Using iTunes' "Show Duplicate Items" feature, you can locate and manually remove duplicate songs on your iTunes music library. Once the library is cleaned, you need only sync iTunes with your iPod to remove duplicates from your device as well. This guide takes iTunes 12 to remove song duplicates.
In iTunes, click "View > Show Duplicate Items" in Music module;
Compare the listed song duplicates upon artist, album, date added, genre, play count, size, bit rate, and more to determine which item to keep and which item to remove;
Hold the "Ctrl" key and click each duplicate you wish to delete.
Connect your iPhone 6 to PC, click your iPhone from the device list, hit "Music" and select "Sync" to sync your library using your existing sync settings.
Connect iPod touch to the computer you normally sync with.
In iTunes, select iPod touch in the sidebar and click the Summary tab.
Click Restore to reinstall the iPod touch software, restore its default settings, and delete data stored on iPod touch. In iTunes, you can also restore from a backup without deleting data stored on iPod touch.
Solution 1. Go to iTunes, go to Edit, Select All, go to Edit once again, select Delete. This will clear your whole music library. Connect you iPod and let it sync. It will delete everything in your iPod. The problem with this is that it will delete all your music in iTunes as well so you better back it up elsewhere.
Solution 2. Go to iTunes, connect your iPod, let it sync. Do not disconnect your iPod. On the left hand side of the screen you will see "Library", "Store", "Devices", etc. Go to "Devices" and you will see your iPod's name there. Click on it and you will see on the right hand side of your screen your iPod, with some menus tabs. On the first tab (Summary), make sure that "Sync only checked songs" is activated. Then go to the second tab ("Music"). Make sure "Sync music" is activated and "Selected playlists" is also activated. Make sure NONE of the playlists is activated. At the bottom right hand side of the scree there is a button that says "Sync". Press it and it will sync no songs into your iPod. That should clear the songs but leave the contents in iTunes intact. If you want to put some playlists in your iPod, then check only those and only those will be added to your iPod.
It is normal for it to take a while before it syncs. If you want it to be faster, make sure you save files to be synced with your Ipod on your hard disk. And make sure to download latest Itunes with quicktime and also update your ipod software.
If this still does not work. Try to uninstall Itunes and then re-install.
ok i think i know what you mean. i had the sme problem. first totally remove all quicktime and iTunes. then go back to apple.com and download iTunes. Quicktime should install with it. Or it should pop up saying if you want to.
go to itunes.com and dl itunes + quicktime. install and scan pc for songs if u already have songs, otherwise, go to the itunes music store in itunes and buy + dl some musin. plug the cable into your ipod and computer, and transfer